Elsevier, Materials Today Sustainability, Volume 9, September 2020
Solar light-driven water splitting provides a promising way to store and use abundant solar energy in the form of gaseous hydrogen which is the cleanest chemical fuel for mankind; therefore this field has been attracting increasing attention over the past decades.
The two-dimensional (2D) ultrathin Mg-Al layered double hydroxide modified by magnetic Fe3O4 (Fe3O4/Mg-Al LDH) was successfully synthesized via the co-precipitation method. The Fe3O4/Mg-Al LDH not only exhibits superior separation efficiency of charge carriers but also possesses signally enhanced photocatalytic activity for CO2 reduction than Mg-Al LDH. The as-prepared Fe3O4/Mg-Al LDH affords the CO and CH4 generation rate of 442.2 µmol g−1 h−1 and 223.9 µmol g−1 h−1. The enhanced reduction CO2 activity mainly comes from synergetic effect of Fe3O4 and ultrathin Mg-Al LDH.
The detection of pharmaceuticals and endocrine disrupting compounds (EDCs), known as emerging contaminants (ECs), in the environment has attracted growing concern due to their toxicity and potential hazard to the ecosystems and humans. These contaminants are consumed at high quantities worldwide and they are released deliberately or accidentally into the water resources. The conventional treatment technologies that use biological processes cannot effectively remove these contaminants.